唐幸福

教授

Tel:021-65642997

Email:tangxf@fudan.edu.cn

研究方向:生态环境,环境催化,大气污染控制,环境功能材料

个人简历

教育简历

  • 2003.09-2006.06, 中国科学院大连化学物理研究所,催化基础国家重点实验室,博士

  • 2000.09-2003.06, 广西师范大学,化学系,硕士

工作简历

  • 2014.12-至今  复旦大学,环境科学与工程系,教授、博导

  • 2012.07-2014.11  复旦大学,环境科学与工程系,副教授、博导

  • 2013.08-2013.09  University of California, Los Angeles, 物理与天文学院,访问教授

  • 2012.04-2013.04  Delft University of Technology, 催化工程中心,访问学者

  • 2008.07-2012.06  复旦大学,环境科学与工程系,副教授、硕导

  • 2006.09-2008.6  清华大学,环境学院,博士后

博士生导师/方向

  • 大气污染物氮氧化物的选择性催化还原

  • 催化控制挥发性大气有机污染物

  • 天然气无污染催化燃烧利用技术

  • 大气界面化学和环境催化基础理论

荣誉与奖励

  • 2017年,上海市自然科学奖,二等奖,排名1

  • 2012年获得教育部“新世纪优秀人才支持计划”。

人才培养

本科生课程:

  • 《有机化学》

科学研究

主持和参与的主要项目/课题

  • 国家自然科学基金,低温分解硫酸氢铵的氨选择性还原氮氧化物催化剂,2020-2023,66万,主持 (No.21976037)

  • 国家自然科学基金,负载型金属单原子催化剂低温去除气态苯,2018-2021,66万,主持 (No.21777030)

  • 国家自然科学基金,强抗碱金属中毒的氨选择性还原氮氧化物催化剂,2015-2018,88万,主持 (No.21477023)

  • 上海市重点基金,生物质燃烧氮氧化物(NOx)排放控制技术的研究,2014-2017,60万,主持 (14JC1400400)

  • 中荷合作交流基金,Addressing the future de-NOx Catalysis: Alkali-resistant Biomass (Co-)Fuelled Power Plants,2013-2015,37万,主持  (No. 13CDP013)

  • 教育部新世纪优秀人才支持计划,大气污染控制化学,2013-2015,50万,主持  (No. NCET-12-0131)

  • 国家自然科学基金,单原子金属催化活性中心低温完全氧化甲醛,2013-2015,50万,主持  (No.21277032)

  • 国家自然科学基金,抗硫疏水性锰分子筛低温氨选择性还原氮氧化物,2011-2013,35万,主持  (No.21077026)

  • 国家自然科学基金,纳米氧化锰分子筛低温去除甲醛的研究,2010-2012,32万,主持  (No.20977018)

  • 教育部高校博士点基金,催化去除甲醛关键技术和反应机理的研究,主持  (No. 20090071120005)

  • 上海市自然科学基金:氧化锰分子筛低温控制氮氧化物技术的研究  (No. 09ZR1402500)

教研成果

研究成果:

  • 1. 高效脱硝技术

构建了碱金属离子交换-配位型中毒机理,发明了强抗碱金属中毒的高效脱硝催化剂,突破了传统脱硝催化剂应用于高碱或碱土金属燃煤或生物质燃料烟气脱硝技术的一个重要瓶颈;相关成果被美国化工新闻杂志Chemical & Engineering News专题报道,同时被美国环保汽车会网Green Car Congress报道。

图1. Chemical & Engineering News的专题报道

  • 2. 催化去除VOCs技术

创建了“反Ostwald合成单原子催化剂”的机理,建立了原子分散金属银催化剂的合成方法,突破了传统的金属纳米粒子在热作用下烧结的生长机理,使金属的利用率获得了最高的原子经济性;相关成果被Nature China栏目以Research Highlights的形式报道。

图2. Nature China的Research Highlights报道

  • 3. 环境催化基本原理

确定了一种高活性的二氧化锰催化剂在SCR反应中的催化活性位(Catalytically Active Sites),对SCR反应的机理研究和高效SCR催化剂的设计开发具有重要的意义;相关成果相继被国际著名的ChemistryViews网站以Highlights的形式报道,同时被Angew. Chem. Int. Ed杂志以Spotlights的形式报道(Angew. Chem. Int. Ed. 2015, 54, 7740-7743)。

图3. ChemistryViews网站的Highlights报道

代表性论文:

  • Yaxin Chen, Daiming Tang, Zhiwei Huang, Xi Liu, Jun Chen, Takashi Sekiguchi, Weiye Qu, Junxiao Chen, Dongrun Xu, Yoshio Bando, Xiaolei Hu, Xiaoping Wang, Dmitri Golberg & Xingfu Tang*. Stable single atomic silver wires assembling into a circuitry-connectable nanoarray. Nat Commun. 2021, 12, 1191.

  • Xiaolei Hu, Junxiao Chen, Weiye Qu, Rui Liu, Dongrun Xu, Zhen Ma, and Xingfu Tang*. Sulfur-Resistant Ceria-Based Low-Temperature SCR Catalysts with the Non-bulk Electronic States of Ceria. Environ. Sci. Technol. 2021, 55, 8, 5435-5441.

  • Weiye Qu, Xiaona Liu, Junxiao Chen, Yangyang Dong, Xingfu Tang* & Yaxin Chen*.  Single-atom catalysts reveal the dinuclear characteristic of active sites in NO selective reduction with NH3. Nat. Commun. 2020, 11, 1532.

  • Yaxin Chen, Chao Li, Junxiao Chen, and Xingfu Tang* Self-Prevention of Well-Defined-Facet Fe2O3/MoO3 against Deposition of Ammonium Bisulfate in Low-Temperature NH3-SCR. Environ. Sci. Technol. 2018, 52, 11796-11802.

  • Junxiao Chen, Yaxin Chen, Meijuan Zhou, Zhiwei Huang, Jiayi Gao, Zhen Ma, Jianmin Chen, and Xingfu Tang*. Enhanced Performance of Ceria-Based NOx Reduction Catalysts by Optimal Support Effect. Environ. Sci. Technol. 2017, 51, 473-478.

  • Weiye Qu, Yaxin Chen, Zhiwei Huang, Jiayi Gao, Meijuan Zhou, Junxiao Chen, Chao Li, Zhen Ma, Jianmin Chen, and Xingfu Tang*. Active tetrahedral iron sites of γ‑Fe2O3 catalyzing NO reduction by NH3. Environ. Sci. Technol. Lett. 2017, 4, 6, 246-250.

  • Yaxin Chen, Zhiwei Huang, Meijuan Zhou, Zhen Ma, Jianmin Chen, and Xingfu Tang* Single silver adatoms on nanostructured manganese oxide surfaces: boosting oxygen activation for benzene abatement. Environ. Sci. Technol. 2017, 51, 2304-2311.

  • YaxinChen, ZhiweiHuang, XiaoGu, ZhenMa, JianminChen, XingfuTang*. Top-down synthesis strategies: Maximum noble-metal atom efficiency in catalytic materials. Chinese. J. Catal., 2017, 38, 1588.

  • Yaxin Chen, Jiayi Gao, Zhiwei Huang, Meijuan Zhou, Junxiao Chen, Chao Li, Zhen Ma, Jianmin Chen, and Xingfu Tang*. Sodium Rivals Silver as Single-Atom Active Centers for Catalyzing Abatement of Formaldehyde. Environ. Sci. Technol. 2017, 51, 12, 7084-7090.

  • Li Zheng, Meijuan Zhou, Zhiwei Huang, Yaxin Chen, Jiayi Gao, Zhen Ma, Jianmin Chen, and Xingfu Tang*. Self-Protection Mechanism of Hexagonal WO3-Based DeNOx Catalysts against Alkali Poisoning. Environ. Sci. Technol. 2016, 50, 11951-11956.

  • Yaxin Chen, Guangkai Tian, Meijuan Zhou, Zhiwei Huang, Chenxi Lu, Pingping Hu, Jiayi Gao, Zhaoliang Zhang*, and Xingfu Tang*. Catalytic Control of Typical Particulate Matters and Volatile Organic Compounds Emissions from Simulated Biomass Burning. Environ. Sci. Technol. 2016, 50, 5825-5831.

  • Yaxin Chen, Zhiwei Huang, Meijuan Zhou, Pingping Hu, Chengtian Du, Lingdong Kong, Jianmin Chen and  Xingfu Tang*. The active sites of supported silver particle catalysts in formaldehyde oxidation. Chem. Commun., 2016, 52, 9996-9999.

  • Zhiwei Huang, Hao Li, Jiayi Gao, Xiao Gu, Li Zheng, Pingping Hu, Ying Xin, Junxiao Chen, Yaxin Chen, Zhaoliang Zhang, Jianmin Chen, and Xingfu Tang*. Alkali- and Sulfur-Resistant Tungsten-Based Catalysts for NOx Emissions Control. Environ. Sci. Technol. 2015, 49, 14460-14465.

  • Pingping Hu, Zhiwei Huang, Xiao Gu, Fei Xu, Jiayi Gao, Yue Wang, Yaxin Chen, and Xingfu Tang*. Alkali-Resistant Mechanism of a Hollandite DeNOx Catalyst. Environ. Sci. Technol. 2015, 49, 7042-7047.

  • Fei Xu, Zhiwei Huang, Pingping Hu, Yaxin Chen, Lei Zheng, Jiayi Gao, Xingfu Tang*. The promotion effect of isolated potassium atoms with hybridized orbitals in catalytic oxidation. Chem. Commun., 2015, 51, 9888-9891.

  • Pingping Hu, Zakariae Amghouz, Zhiwei Huang, Fei Xu, Yaxin Chen, and Xingfu Tang*. Surface-Confined Atomic Silver Centers Catalyzing Formaldehyde Oxidation. Environ. Sci. Technol. 2015, 49, 2384-2390.

  • Pingping Hu, Manfred Erwin Schuster, Zhiwei Huang, Fei Xu, Shifeng Jin, Yaxin Chen, Weiming Hua, Dang Sheng Su, Xingfu Tang*. The Active Sites of a Rod‐Shaped Hollandite DeNOx Catalyst. Chem. Eur.J.2015, 21, 9619-9623.

  • Yaxin Chen, Takeshi Kasama, Zhiwei Huang, Pingping Hu, Jianmin Chen, Xi Liu, Xingfu Tang*. Highly Dense Isolated Metal Atom Catalytic Sites: Dynamic Formation and In Situ Observations. Chem. Eur.J.2015, 21, 17397-17402.

  • Pingping Hu, Zhiwei Huang, Zakariae Amghouz, Michiel Makkee, Fei Xu, Freek Kapteijn, Alla Dikhtiarenko, Yaxin Chen, Xiao Gu, and Xingfu Tang*. Electronic Metal–Support Interactions in Single-Atom Catalysts. Angew. Chem. 2014, 126, 3486-3489.

  • Zhiwei Huang, Xiao Gu, Wen Wen, Pingping Hu, Michiel Makkee, He Lin, Freek Kapteijn, Xingfu Tang*. A “Smart” Hollandite DeNOx Catalyst: Self‐Protection against Alkali Poisoning. Angew. Chem. Int. Ed. 2013, 52, 660-664.

  • Zhiwei Huang, Xiao Gu, Qingqing Cao, Pingping Hu, Jiming Hao, Junhua Li, Xingfu Tang*. Catalytically Active Single‐Atom Sites Fabricated from Silver Particles. Angew. Chem. Int. Ed. 2012, 51, 4198-4203.

更多论文成果详见以下链接:http://www.researcherid.com/rid/J-3309-2013